Emery has been without a club since being sacked as Arsenal boss in November and replaces Javier Calleja at Villarreal.
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Villarreal will hire Unai Emery as their next manager, sources confirmed to ESPN.
Real Madrid secured their 34th league title -- and first since 2017 -- with a victory over Villarreal on Thursday.
Zinedine Zidane risked tarnishing his record by diving back into the Real Madrid job 10 months but he has proved the perfect man for the job.
Villarreal's hopes of finishing in La Liga's top four ended with a 2-1 defeat at home to Real Sociedad.
Villarreal won 3-1 away to Getafe in La Liga following a glut of goals in the second half to maintain their push for a Champions League spot.
Barcelona defeated Villarreal 4-1 to keep pace with Real Madrid in the La Liga standings.
Villarreal beat neighbours Valencia 2-0 on Sunday with a pair of brilliant volleyed goals to boost their chances of a top-four finish.
Sharp shooting allowed Sevilla to twice come from behind and take a valuable away point in a 2-2 draw at in-form Villarreal on Monday.
Villarreal kept alive their hopes of claiming a Europa League qualifying berth after beating Mallorca 1-0.
Villarreal midfielder Manu Trigueros scored a late winner to give his side a 1-0 La Liga away victory at relegation-threatened Celta Vigo.
Atletico Madrid's record signing Joao Felix scored for the first time in the league for almost five months as his side beat Villarreal 3-1 at home o
Real Sociedad's hopes of getting back into La Liga's top four were hit as they slumped to a 2-1 defeat at home to Villarreal on Sunday.
Atletico Madrid's problems deepened as they were held to a 0-0 draw at Villarreal in La Liga on Friday, stretching their winless run to four games.
A judge in Madrid turned down on Friday La Liga's request to stage Villarreal's home league game against Atletico Madrid on Dec. 6 in Miami.
The Royal Spanish Football Federation has received a letter from Real Madrid opposing playing a regular season La Liga game in the United States.
Villarreal's president has confirmed he is in talks with La Liga in a bid to stage his team's Dec. 8 league game against Atletico Madrid in Miami.
The Spanish Football Federation (RFEF) has released a statement condemning a VAR decision during Valencia's 1-0 victory against Athletic Bilbao.
Barcelona secured a much-needed 2-1 victory at home to Villarreal in La Liga on Tuesday but Lionel Messi's removal cast a cloud.
Gareth Bale scored two goals as Real Madrid came back twice to earn a draw at Villarreal in La Liga action on Sunday.
Villarreal winger Samuel Chukwueze's deal with music mogul Jay-Z's Roc Nation management company catapulted the Nigeria player into the spotlight.